A Vault Owner is not able to edit the Portal User permission set in Vault.
System managed permission sets cannot be modified in Vault.
The Portal User permission set is a system managed permission set, that cannot be modified by any Vault user. A workaround for this would be to;
- Make a copy of the Portal User permission set.
- Modify the new permission set to the desired requirements.
- Assign the newly created permission set to the desired users.
Vault Help Documentation: How to create Security Profiles by Copying
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